head to head
Neither is simply harder - they are hard in different places. Crayon Physics Deluxe demands more variance; Portal demands more execution.

Optimization · Pure Optimization
Draw crayon shapes that become physics objects to roll a ball to a star.

Optimization · Pure Optimization
The portal-gun puzzle game whose solutions are everything.
Crayon Physics Deluxe leans Optimization (Pure Optimization); Portal leans Optimization (Pure Optimization).
Portal leans clearly harder on execution.
Crayon Physics Deluxe
Freehand drawing needs only rough motor control
Portal
Portal placement timing modest.
Same score on reads - which means the number cannot separate them. The difference is in what each one asks of you.
Crayon Physics Deluxe
No opponent exists
Portal
No adversary modeling player.
Crayon Physics Deluxe leans clearly harder on variance.
Crayon Physics Deluxe
Physics wobble makes contraptions slightly unpredictable
Portal
Deterministic chambers; no randomness.
Same score on optimization - which means the number cannot separate them. The difference is in what each one asks of you.
Crayon Physics Deluxe
Each level rewards inventing an efficient contraption
Portal
Pure puzzle-solving optimization.
A matching score does not mean a matching test. Two games can both sit at 10 on execution and demand completely different things of you - which is why the reasoning above matters more than the number beside it.